Greg,
Right now, you have a machine in good mechanical state. The only problem you have with this machine is the controller. My advice, do not remove or dismantle any component at this stage.
1-Gather the manuals wiring diagrams and any information you can find.
2-Study the servo drive CONTROL METHOD (analog, digital, industrial communication bus etc …)
3- Study existing wiring diagrams and determine the number and type of IO’s (sourcing/sinking)
4- study the type of controller you will need, the type of daughter boards needed and type of PC (pci/pcie/ethernet/Mitsubishi bus communication bus … etc
5- Modify the existing wiring diagrams to reflect the changes required. Keep in mind that the machine was designed and assembled by highly skilled craftsmen, at this stage you will focus on keeping the modifications to existing components to a strict minimum.
6- With all the above knowledge and mods you will be ready to configure the controller and choose GUI
Note: machine integration requires patience especially if you have not done it before on a machine such as vmc. (Bounding, grounding, shielding can be nightmare, modifying the safety control system can become a liability and changing from sourcing/sinking io can be laborious, etc …), keep it simple stupid (KISS) is the answer to a successful project.